Nii Share definition Flag (N.)A derivitive from the Japanese language. It is translated to be "Brother." or "Older-brother." Nii, give me back my toy! Nii, your the bestest brother a kid could have. Nii by BlackBlood Sky July 21, 2011 0 0 Get merch Get the Nii mug. Buy Now — $32.95 See more merch