Steming from the term "Crazy", when Referring to someone as "Cray Cray", signifies their craziness to a whole other level. The ultimate second power of crazy. This person can either be insane in the brain. Or simply, TOO DOWN. To the point where its not even cool anymore.
Boy: "Lets have a milk chugging contest"
Girl: "Ok No. Don't get cray cray."
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