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1.
1)The act of "Balling" in the video game Pokémon.

2)Knowing a lot about Pokémon and being a prick about it.
Billy: Wow look at Chen over there! He sure is Poké Ballin' with his Dugtrio!

Chen: Actually it's a Dodrio, RETARD!

Jeff: Yeah Chen sure is Poké Ballin' today.
by darthlazlo October 07, 2010
 
2.
When you hit your partner in the face with your balls and scream "GOTTA CATCH 'EM ALL!!!"
Phil was Pokeballin' Shannon while she was she was watching Digimon.
by Pokeballin' November 13, 2009